MLS Research
Extra-tropical Strat-Trop Exchange
Contact Gloria Manney
Understanding dynamical, transport and chemical processes in the extra-tropical (ET) upper troposphere and lower stratosphere (UTLS) is critical to advancing climate change and pollution transport studies.
For example, water vapor and ozone are both key greenhouse gases in the UTLS, and their distributions are strongly affected by stratosphere-troposphere exchange processes. In the lowermost stratosphere (the portion of the extratropics where some part of the lower latitude region is in the troposphere), there is a complex interplay of stratospheric (e.g., chemical ozone loss) and tropospheric (e.g., pollution generation and transport, fire-related convection) processes, and intrusions of stratospheric air into the troposphere and vice versa are common.
The coupled chemistry and climate of the UTLS respond to both tropospheric climate change [e.g. Santer et al., 2004; WMO, 2007] and to O3 depletion in the lower stratosphere (link to polar processes section) [e.g., Seidel and Randel, 2006]; the complexity of causes of tropopause-level changes makes our ability to accurately detail UTLS variability especially critical. Both radiative forcing and surface temperature are most sensitive to O3 changes near the tropopause [e.g., Forster and Shine, 1999].
Radiative effects of water vapor near the ET tropopause have been shown to be instrumental in determining the thermal structure in the UTLS [e.g., Randel 2007]. Upper tropospheric winds (the jet streams whose tops extend into the lowermost stratosphere) and tropopause characteristics have been shown to be sensitive to climate change [e.g., Lorenz and DeWeaver, 2007; Archer and Caldeira, 2008].
The Antarctic O3 hole has caused significant temperature changes in the lower stratosphere; a significant part of the ozone depletion occurs in the sub-vortex (the lowest part of the polar vortex that extends into the lowermost stratosphere), where it can be more efficiently transported to midlatitudes and possibly into the troposphere.
Changes in the Brewer-Dobson Circulation (the large-scale seasonally varying circulation of the stratosphere), synoptic eddies (storms) in the upper troposphere, and midlatitude convection are expected to alter the extent and consequences of ET stratosphere-troposphere exchange.
Pollution products transported from the troposphere up into the lower stratosphere influence ozone chemistry there [e.g. Hegglin et al., 2006; WMO, 2007]; conversely, stratospheric O3 transported down also influences tropospheric chemistry [e.g., WMO, 2007; Hsu and Prather, 2009].
Until recent years, most satellite measurements did not extend down into the ET UTLS, and studies of the ET UTLS were primarily limited to analysis of sporadic and sparse (albeit very high spatial and temporal resolution) aircraft data.
With the launch of the Aura satellite, MLS provides measurements of O3, HNO3, CO and H2O, as well as temperature, covering the lowermost stratosphere with global daily coverage; other measurements (e.g., HCl and ClO) extend into the upper part of this region.
Meteorological analyses from advanced data assimilation systems (DAS) provide comprehensive information on the jet streams (the winds that control transport and mixing of trace gases), tropopause variations, and temperature structure in the UTLS, that is, the dynamical factors that control trace gas transport and influence chemical processes.
Studies using MLS data, in conjunction with DAS analyses and high resolution but sparse aircraft data, can contribute to advancing our understanding of the ET UTLS and its role in climate change processes.
MLS-related publications related to extra-tropical stratosphere-troposphere exchange
Rawat, P., M. Naja, E. Fishbein, P. Thapliyal, R. Kumar, P. Bhardwaj, A. Jaiswal, S. Tiwari, S. Venkataramani and S. Lal
Performance of AIRS ozone retrieval over the central Himalayas: Case studies of biomass burning, downward ozone transport and radiative forcing using long-term observations
Vogel, A., J. Ungermann and H. Elbern
Analyzing trace gas filaments in the Ex-UTLS by 4D-variationalassimilation of airborne tomographic retrievals
Blunden, J. and T. Boyer
State of the Climate in 2021
Fazel-Rastgar, F. and V. Sivakumar
A severe weather system accompanied by a stratospheric intrusion during unusual warm winter in 2015 over the South Africa: An initial synoptic analysis
Fujiwara, M., G.L. Manney, L.J. Gray and J.S. Wright
SPARC Reanalysis Intercomparison Project S-RIP Final Report
n/a 2022Li, D., J. Bian, X. Zhang, B. Vogel, R. Müller and G. Günther
Impact of typhoon Soudelor on ozone and water vapor in the Asian monsoon anticyclone western Pacific mode
Martinsson, B., J. Friberg, O. Sandvik and M. Sporre
Five-satellite-sensor study of the rapid decline of wildfire smoke in the stratosphere
Pan, L., D. Kinnison, Q. Liang, M. Chin, M. Santee, J. Flemming, W. Smith, S. Honomichl, J. Bresch, L. Lait, Y. Zhu, S. Tilmes, P. Colarco, J. Warner, A. Vuvan, C. Clerbaux, E. Atlas, P. Newman, T. Thornberry, W. Randel and O. Toon
A Multimodel Investigation of Asian Summer Monsoon UTLS Transport Over the Western Pacific
Peng, K., J. Luo, J. Mu, X. Cao, H. Tian, L. Shang and Y. Guo
Impact of intensity variability of the Asian summer monsoon anticyclone on the chemical distribution in the upper troposphere and lower stratosphere
Qie, K., W. Wang, W. Tian, R. Huang, M. Xu, T. Wang and Y. Peng
Enhanced upward motion through the troposphere over the tropical western Pacific and its implications for the transport of trace gases from the troposphere to the stratosphere
Salawitch, R. and L. McBride
Australian wildfires depleted the ozone layer
Santee, M.L., A. Lambert, G.L. Manney, N.J. Livesey, L. Froidevaux, J.L. Neu, M.J. Schwartz, L.F. Millán, F. Werner, W.G. Read, M. Park, R.A. Fuller and B.M. Ward
Prolonged and Pervasive Perturbations in the Composition of the Southern Hemisphere Midlatitude Lower Stratosphere From the Australian New Year's Fires
Xiong, X., X. Liu, W. Wu, K.E. Knowland, Q. Yang, J. Welsh and D. Zhou
Satellite observation of stratospheric intrusions and ozone transport using CrIS on SNPP
Babu, S.R., M.V. Ratnam, G. Basha, S. Pani and N. Lin
Structure, dynamics, and trace gas variability within the Asian summer monsoon anticyclone in the extreme El Niño of 2015–2016
Blunden, J. and T. Boyer
State of the Climate in 2020
Bossolasco, A., F. Jegou, P. Sellitto, G. Berthet, C. Kloss and B. Legras
Global modeling studies of composition and decadal trends of the Asian Tropopause Aerosol Layer
Emmanuel, M., S.V. Sunilkumar, M. Muhsin, P.R.S. Chandran, K. Parameswaran, B.S. Kumar, A. Maitra, A.N.V. Satyanarayana and N. Nagendra
Effect of monsoon dynamics and deep convection on the upper troposphere lower stratosphere water vapour over Indian monsoon region
Fujiwara, M., T. Sakai, T. Nagai, K. Shiraishi, Y. Inai, S. Khaykin, H. Xi, T. Shibata, M. Shiotani and L. Pan
Lower-stratospheric aerosol measurements in eastward-shedding vortices over Japan from the Asian summer monsoon anticyclone during the summer of 2018
Gharibzadeh, M., A. Bidokhti and K. Alam
The interaction of ozone and aerosol in a semi-arid region in the Middle East: Ozone formation and radiative forcing implications
He, X., J. Luo, X. Xu, L. Ren, H. Tian, L. Shang and P. Xu
The QBO Modulation on CO Distribution in the UTLS Over the Asian Monsoon Region During Boreal Summer
Jenkins, G., V.D. Castro, B. Cunha, I. Fontanez and R. Holzworth
The Evolution of the Wave‐One Ozone Maximum During the 2017 LASIC Field Campaign at Ascension Island
Karpowicz, B., W. McCarty and K. Wargan
Investigating the utility of hyperspectral sounders in the 9.6 μm band to improve ozone analyses
Kumar, K., B. Singh and Kumar, K.
Intriguing aspects of Asian Summer Monsoon Anticyclone Ozone variability from Microwave Limb Sounder measurements
Park, M., H. Worden, D. Kinnison, B. Gaubert, S. Tilmes, L. Emmons, M. Santee, L. Froidevaux and C. Boone
Fate of pollution emitted during the 2015 Indonesian Fire Season
Plaza, N., A. Podglajen, C. Peña-Ortiz and F. Ploeger
Processes influencing lower stratospheric water vapour in monsoon anticyclones: insights from Lagrangian modelling
Pumphrey, H., M. Schwartz, M. Santee, G. Kablick III, M. Fromm and N. Livesey
Microwave Limb Sounder MLS observations of biomass burning products in the stratosphere from Canadian forest fires in August 2017
Rieger, L.A., W.J. Randel, A.E. Bourassa and S. Solomon
Stratospheric Temperature and Ozone Anomalies Associated With the 2020 Australian New Year Fires
Tang, Q., M. Prather, J. Hsu, D. Ruiz, P. Cameron-Smith, S. Xie and J. Golaz
Evaluation of the interactive stratospheric ozone O3v2 module in the E3SM version 1 Earth system model
Wang, M. and Q. Fu
Stratosphere‐Troposphere Exchange of Air Masses and Ozone Concentrations Based on Reanalyses and Observations
Barret, B., E. Emili and E.L. Flochmoen
A tropopause-related climatological a priori profile for IASI-SOFRID ozone retrievals: improvements and validation
Blunden, J. and D.S. Arndt
State of the Climate in 2019
Fadnavis, S., C. Sioris, N. Wagh, R. Chattopadhyay, M. Tao, P. Chavan and T. Chakroborty
A rising trend of double tropopauses over South Asia in a warming environment: Implications for moistening of the lower stratosphere
Girach, I., P. Nair, N. Ojha and L. Sahu
Tropospheric carbon monoxide over the northern Indian Ocean during winter: influence of inter-continental transport
Honomichl, S. and L. Pan
Transport From the Asian Summer Monsoon Anticyclone Over the Western Pacific
Itahashi, S., R. Mathur, C. Hogrefe and Y. Zhang
Modeling stratospheric intrusion and trans-Pacific transport on tropospheric ozone using hemispheric CMAQ during April 2010 -- Part 1: Model evaluation and air mass characterization for stratosphere-troposphere transport
Khaykin, S., B. Legras, S. Bucci, P. Sellitto, L. Isaksen, F. Tencé, S. Bekki, A. Bourassa, L. Rieger, D. Zawada, J. Jumelet and S. Godin-Beekmann
The 2019/20 Australian wildfires generated a persistent smoke-charged vortex rising up to 35 km altitude
Miyazaki, K., K. Bowman, K. Yumimoto, T. Walker and K. Sudo
Evaluation of a multi-model, multi-constituent assimilation framework for tropospheric chemical reanalysis
Qu, Z., Y. Huang, P. Vaillancourt, J. Cole, J. Milbrandt, M. Yau, K. Walker and J.D. Grandpré
Simulation of convective moistening of the extratropical lower stratosphere using a numerical weather prediction model
Robinson, J., A. Kotsakis, F. Santos, R. Swap, K.E. Knowland, G. Labow, V. Connors, M. Tzortziou, N. Abuhassan, M. Tiefengraber and A. Cede
Using networked Pandora observations to capture spatiotemporal changes in total column ozone associated with stratosphere-to-troposphere transport
Schoeberl, M.R., L. Pfister, T. Wang, J. Kummer, A.E. Dessler and W. Yu
Erythemal Radiation, Column Ozone, and the North American Monsoon
Schwartz, M., M. Santee, H. Pumphrey, G. Manney, A. Lambert, N. Livesey, L. Millán, J. Neu, W. Read and F. Werner
Australian New Year's PyroCb Impact on Stratospheric Composition
Uma, K.N., T.S. Mohan and S. Das
Role of Intra-Seasonal Variability in the Indian Summer Monsoon on the Hydration and Dehydration of the Upper Troposphere
Werner, F., M.J. Schwartz, N.J. Livesey, W.G. Read and M.L. Santee
Extreme Outliers in Lower Stratospheric Water Vapor Over North America Observed by MLS: Relation to Overshooting Convection Diagnosed From Colocated Aqua‐MODIS Data
Xu, X., H. Tian, K. Qie, X. He, R. Zhang and H. Tu
A Study on the Trend of the Upper Tropospheric Water Vapor over the Tibetan Plateau in Summer
Yu, W., A. Dessler, M. Park and E. Jensen
Influence of convection on stratospheric water vapor in the North American monsoon region
Blunden, J. and D. Arndt
State of the Climate in 2018
Diallo, M., P. Konopka, M. Santee, R. Müller, M. Tao, K. Walker, B. Legras, M. Riese, M. Ern and F. Ploeger
Structural changes in the shallow and transition branch of the Brewer–Dobson circulation induced by El Niño
Emili, E., B. Barret, E.L. Flochmoën and D. Cariolle
Comparison between the assimilation of IASI Level 2 ozone retrievals and Level 1 radiances in a chemical transport model
Inness, A., M. Ades, A. Agustí-Panareda, J. Barré, A. Benedictow, A. Blechschmidt, J. Dominguez, R. Engelen, H. Eskes, J. Flemming, V. Huijnen, L. Jones, Z. Kipling, S. Massart, M. Parrington, V. Peuch, M. Razinger, S. Remy, M. Schulz and M. Suttie
The CAMS reanalysis of atmospheric composition
Nützel, M., A. Podglajen, H. Garny and F. Ploeger
Quantification of water vapour transport from the Asian monsoon to the stratosphere